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[Sweet and Sour] Vocaloid Unrequited Love Song Collection [Bittersweet]

There are many different forms of unrequited love.

Your heart might race nonstop with your first crush, or ache when you see the person you like talking to someone else…

In this article, we’ve put together a selection of Vocaloid songs about unrequited love—perfect for those of you who are in love right now, or who want to remember how it felt back then.

As mentioned above, everyone has their own version of “unrequited love,” so we’ve picked out a wide variety of love songs!

You’re sure to find a track that perfectly matches your mood!

[Bittersweet] Vocaloid Unrequited Love Song Collection [Heart-wrenching] (61–70)

black catred hair

[GUMI] Black Cat PV English and romaji subs
Black cat, red hair

A song that can only be summed up as “heart-wrenching”! It’s about a girl who’s turned into a black cat and can’t get the person she loves to notice her.

She wants them to turn around, but not only do they never look back—she ends up being forgotten.

It really pierces the heart.

Perfect for when you just want to have a good cry!

Champion Road of LoveNem

Love’s Champion Road / Kagamine Len
Champion Road of Love Nem

A passionate love song that likens romance to a boxing match.

Nem’s “Champion Road of Love” was released in March 2024.

Written specifically for the game “Fit Boxing feat.

Hatsune Miku — Exercise with Miku,” it features Kagamine Len’s powerful vocals.

With brassy sounds and a rhythmic groove, it brilliantly conveys the protagonist’s passion and inner conflict.

The image of a man giving his all to win at love will resonate with anyone ready to take on a new challenge.

The more you listen, the more energized you’ll feel!

Don't be happy.Gray Slumber

A delicately drawn, heart-wrenching Vocaloid song that captures the ache of unrequited love.

Released by Nemuri Haiiro in February 2024, the track features Nurse-robot_Type T’s airy, whispery vocals that leave a strong impression.

While wishing for the other person’s happiness, the lyrics also reveal a conflicting desire for them not to leave—an emotional complexity that seeps through every line.

Many listeners will relate to the words where love and dependence intersect.

A definitive anthem of one-sided love, painting a bittersweet yet tender form of romance.

Perfect for those struggling with love or reminiscing about past relationships.

Life is short, fall in love, young maiden.Death Ohagi

"Life is short, fall in love, girls" – Death Ohagi feat. Kasane Teto
Life is short—fall in love, maiden. Death ohagi.

It’s not just about unrequited love—it’s a song brimming with pure life energy.

It portrays the entire life of a girl who ran away from home, all through the theme of love.

The phrase “Life is short, fall in love, young maiden” is often used, but this song is precisely the one most deserving of those words.

Unrequited Love SambaOwata-P

[Hatsune Miku] Unrequited Love Samba [DIVA Submission Song]
Unrequited Love Samba Owata-P

As the title suggests, it’s a samba-style, high-tempo track.

Beyond the lyrics, the sound captures the fluttery excitement of being in love and that slightly flustered feeling, too.

It makes you want to dance along, doesn’t it?

First Love CiderVitamin Aniki ♂

As the title suggests, the lyrics capture the bursting feelings of unrequited love, perfectly matched by Hatsune Miku’s girlish vocals.

It’s a mid-tempo guitar rock track that fills you with excitement as you listen.

Highly recommended for anyone in the thick of their youth.

Transparent in summerTwinfield

Transparent in Summer / Twinfield feat. Hatsune Miku
Transparent Twinfield in summer

A refreshing love song wrapped in the transparency of summer.

Released in 2024 by Twinfield, this piece stands out with its crystal-clear melodic lines and shimmering sound.

Centered on themes of summer memories and secret feelings of love, its sentimental lyrics tighten the heart.

Give it a listen, and it will surely carry a fresh, cleansing breeze into yours.