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[Sweet and Sour] Vocaloid Unrequited Love Song Collection [Bittersweet]

There are many different forms of unrequited love.

Your heart might race nonstop with your first crush, or ache when you see the person you like talking to someone else…

In this article, we’ve put together a selection of Vocaloid songs about unrequited love—perfect for those of you who are in love right now, or who want to remember how it felt back then.

As mentioned above, everyone has their own version of “unrequited love,” so we’ve picked out a wide variety of love songs!

You’re sure to find a track that perfectly matches your mood!

[Bittersweet] Vocaloid Unrequited Love Song Collection [Heart-wrenching] (41–50)

Let's go to an alien planet.Iyowa

Let's go to an alien planet / Iyowa feat. Seikai (Take you to an alien / Iyowa feat. Seikai)
Let's go to an alien planet, Neiyowa.

Vocaloid producer Iyowa, known for the smash hit signature song “Kyuukurarin,” captivates listeners with uniquely thematic tracks.

“Let’s Go to Another Planet,” created in 2022, portrays a bittersweet love story.

Its lyrics unfold within a cosmic, UFO-themed world that pairs perfectly with bright, poppy synth tones.

You’ll find solace in the starry vocals that convey feelings both aching and cute.

It’s an unrequited love song with a subtly thrilling vibe—highly recommended for sleepless nights spent thinking about someone you love.

[Bittersweet] Vocaloid Unrequited Love Song Collection [Heart-wrenching] (51–60)

milk teaspoiled tantrum

[Hatsune Miku Append] Milk Tea [Original PV]
It's milk tea, dada.

Love at first sight, and an unrequited love that stayed that way.

It’s a cute yet bittersweet song about a relationship that would make anyone watching feel impatient.

Though it began with love at first sight and no connection between them, everything started from a cup of milk tea.

The happy days that followed for the two warm our hearts as we watch them.

And it’s milk tea again that brings back those days that have now slipped into the past.

It’s a song that takes our emotions for a spin.

LeiaYuyoyuppe

[Megurine Luka] Leia – Remind [Original]
Leia yuyoyuppe

It’s a slightly abnormal track.

The aggressive rock sound is striking above all.

The lyrics, which evoke the image of dragging something beautiful down with your own hands, really hit home.

Recommended for those who want something with a different vibe from a pure love song.

picture book of first loveHONEY WORKS

┗|∵|┓ First Love Picture Book -arrangement- / HoneyWorks feat. GUMI
First Love Picture Book HONEYWORKS

A bittersweet, heart-wrenching Vocaloid song about a love that ended as unrequited.

It’s a track by HoneyWorks (a.k.a.

Haniwa), released in 2011.

By the way, the video is a different arrangement version that was published in 2013.

Given its content, it might especially resonate with working adults.

Listening to it inevitably brings back memories of past love.

At the same time, it’s also a song that gives you the courage to share your feelings.

If you’re a student right now, I hope you experience a love you won’t regret!

Summer’s Collapse, Unrequited LoveAotokei

Summer-Collapse Unrequited Love / Aotokei feat. Hatsune Miku Dark
Summer Collapse, Unrequited Love, Blue Sound Clock

It’s a song with a clean melody that feels refreshing like summer.

It sings of the heartache of unrequited love, where the word “if” is used over and over.

Hatsune Miku sings with a trembling voice as if she’s about to cry—it almost makes you tear up, too.

TwinkleJunky

[Tried making a PV] Twinkle [Kagamine Rin]
Twinkle Junky

It’s a refreshing band-sound love song that begins with sparkling synthesizer tones.

Created by Junky, who also wrote “Melancholic” and “Happy Halloween,” it was released in 2011.

The endlessly sweet-and-sour lyrics and melody make your heart flutter! Feelings that were forced into hiding after the other person drew a line in the relationship… yet they overflow no matter what! It’s a wonderful Vocaloid track that makes you hope—without even meaning to—that someday those wishes will reach the one they’re meant for.

Electric AngelYasuo

[Hatsune Miku] Electric Angel [Project DIVA 2nd]
Electric Angel Yasuo

This is a song you can get completely absorbed in when you’re in love.

Many people can relate to the lyrics that think of nothing but that special someone, and it’s sure to make your heart skip a beat! Highly recommended for your first love in particular! It’s a Vocaloid song that has been beloved for a long time since its release.